By Jean-Louis Salager

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Additional resources for A. Wilhelm Neumann, Robert David, and Yi Zuo (eds): Applied Surface Thermodynamics, 2nd Edition

Sample text

We impose the first condition that all dissipation processes vanish in the composite system by requiring that the total entropy remain fixed. Imposition of the second condition simply requires that the mass of each species remain constant. 54) and normal displacement variations where {Aw,j} denotes the union of all internal surfaces that would intersect the bounding wall during a variation and {Lw,k} denotes the union of all internal contact lines that would intersect the bounding wall during a variation.

Positioning and shifting of dividing surfaces is a matter of practical and theoretical importance; however, the question of the legitimacy of such shifts has often been disregarded. , to coincide, as in Gibbs classical theory, with the position of the surface of tension) is necessary in the generalized theory we may expect greater flexibility from this theory than from the classical one with regards to this choice. It is the purpose of the subsequent sections in this chapter to explore the differences between the two theories and to corroborate further the generalized theory of capillarity.

The Laplace equation of capillarity) in a more direct manner. Only spherical and cylindrical interfacial geometries will be considered for illustration; however, the approach is completely general and applies to any geometry. © 2011 by Taylor and Francis Group, LLC Outline of the Generalized Theory of Capillarity 27 Physically, the particular class of two-phase capillary systems we shall consider is one in which one phase contains a small bubble or droplet of the second phase, either attached to a phase boundary or free.

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